%PDF-1.4 % 1 0 obj <>stream Atypon Systems, Inc.; modified using iText 4.2.0 by 1T3XT 2018-06-05T15:51:19-04:00 Visible Light [2 + 2] Cycloadditions for Reversible Polymer Ligation 10.1021/acs.macromol.8b00613 American Chemical Society David E. Marschner Hendrik Frisch Janin T. Offenloch Bryan T. Tuten C. Remzi Becer Andreas Walther Anja S. Goldmann Pavleta Tzvetkova Christopher Barner-Kowollik application/pdf research-article http://pubs.acs.org/doi/suppl/10.1021/acs.macromol.8b00613 © 2018 American Chemical Society American Chemical Society True © 2018 American Chemical Society © 2018 American Chemical Society Issue 10.1021/acs.macromol.8b00613 VoR 05/09/2018 51 10 3802 3807 © 2018 American Chemical Society article 0024-9297 1520-5835 Macromolecules research-article Issue10.1021/acs.macromol.8b00613VoR endstream endobj 2 0 obj <> endobj 5 0 obj <> endobj 3 0 obj <> endobj 4 0 obj <> endobj 6 0 obj <> endobj 7 0 obj <> endobj 8 0 obj <> endobj 9 0 obj <> endobj 10 0 obj <> endobj 11 0 obj <> endobj 12 0 obj <> endobj 13 0 obj <> endobj 18 0 obj <>/ProcSet[/PDF/Text/ImageC]/ExtGState<>/Font<>/XObject<>/Properties<>>> endobj 15 0 obj <>stream xv$q%f~)$znRJlEɇ,Tv!Pĭ~Z#W_9%DUM i"-#/f.w;=iEZ^dO_% E~t7W'?⶞ߞs+wB;3Sd8]oN~9yԆv9Ha2-¡21gHthuN4i]e1X>~$bk'"qdvסN7"''gD"uYZDr rPrYYshJ*+-Wq^nJD)S&5{EȱP{^uxgE)2RnI5iR9uko~E]X*c(̀klQf֋"\rBY/c!Dڗq  ^Kw yM +KeZC.6$45s.Ot^XɊaEft7N0o(|+\8#bP npG'-s4_iW*{/Ġ]jcudA~>#1~(crB}/dg]]ywu4 MK)Ys_>\NՑw:"c&,IԸ2Ҵ:±ʷ:$b³㱫A9rųմxı°칗<],%1aB[i0E\#7} p/o.8 i̔?EJG2Wz"q`Yg~YT ;O!dl)Y#W~eqT]m-ȹʆ׵Bf|'>σ  _>B[o9/’PG/61(՛?>l~y1:E QF)6/≥vXO6WЋaW_\n?\ Von7gt~KsXW{Tݳ{&-1LYYh !C$Q_%X*.X,U B,-bhWzN#`B…vS\\A*l,(<~u~q}&7(:vZ~¢_\<28'՗|׋ufw5Z~Sr17 q-̭~&<.?looʺf{sAo7W[ඤ?1Ȳt"9K7f<>%zOAj$W_no/n/vwkKͫ^uͽ5K5U1K5V CG_:#UA@1Yy?mn7|)[Cg,#6,O9˜0'|&A 2VdQJ)8ᕛҴ8:b ŔOR4uJ\_[SAg7k]ecj=npʳx͝\oEw۫-+2\|x0kVk0v}`=??q奕nN7꟤3/ ǧ#C'5MO&V:s^=S;Y|s!(~:rcU*Up#·L76:ίR.A||:% e9H>;߼ꌟ2I\[.{ϰ Oٜoo*#'|,k;; E_mﴍj!x AS:[U )`av 'r3`E̷ }W"tZ% o7:4i\Zr--ܠ6(Dijf8{z&~cE:?5T9#%';m u#*>\m^A_[C"}@}':ḀHFiV؉G\,ȝ;r( IDq}=> zm&9.LLzTc u8=z{xxENkK.؀>!a=yz&T[ۻ%((+"}R,ʭ8V[_4UEis;bGnn,CX. 3 WgM K%h݊AOJ*3oċ^Vf6gzB=e^x'W RTؗ[VxEQbn7'%XE}RD\ȹ~+P&& &;] G1a.ˋf*m}v6/k򁪛mr5$jquuG\4q|L_.XV;r>6 yeQ&_~`\W$}&UNrnGk|}LԵ >|ˈXsr_S}vwaˢ=X%q=X kXǽ,C<W2ܞ+k ;(paCy䙨hA(4SH|-{l"h[ߪI^U mi>߿9!>0tp^H6 B G<}-[>R ǧ Rlt=͠s[Ʊf^uZa E#6*yaM^y,w)%υz':[GֺDFQ9=v6W+n50S}~l?\\^j`Zɪ_h&EVYAO|s8oYJMET'j/ -Oͯ~_?[_ D}έ>lL.Tp;]:oRgsP鲪|ާZyCLVm`lANO׀УZ W0")~Vgq6`]tFR9@su-J[ EI撏%1؄!d`h0pmr}!A {ws9n-'qs-Gl z:êÈ 2K/D<郆 u;b[P0~ ˃{X`Ect(y]`-E<7/Hd{΅?}i6s- Vt2;M"}Wߡap]5 A1er_aiB~Nu~T ,#C mlvd liV\V;8qu!轉jyW#rCZ #W[Uت /T[.uE~HGhu#yQY|dSbT ФCT~ Gb ,o7tPV ⺂Ozpx0:j҉y8֣I*2 S;_vo9(v:d^xo;*EAz>q8ʷTDz+-``x]QΕ?BaґQݕx4D.?mgIdϘ B]b (Y`ޑ_]7l9 =.¶KQruUK Mh;uX`Mx-\О]&\]jYIkur~ܒhWីdƵ!zC}ѣn'&8v1Z7wx8b#P =1ж1QK+>|ܼOLA1E 1~Sňoyo7^giњ ?0_|'~ <=bɎ\0[$ٜ̽FZ' Lv6EK F%1C&CO8|m%5%p<0mq%sͧbḉ DiCiwo>)ݳMLյ<5w6́Tb_9rS,P[ˤ ;3 EGH*͌ɩ&K3LK"Gy@ *Sq60<k3фޖ;i&;淯4F?!(bFdY!`GPY=3] \{,[$I)Bh_Pf/Plb!K~Y<8.^anЗ8ީf4Guy[K_n=DvV#w=%jyT(%zjB.i_!jG}XLWp ^fw"wƀBtYde$YjF:߳LÄNá>@϶rJsg' 5P&|跞Ž]è`E ` ͬsA-W`rQ f>ԙ?v0hj~Ww7p"ڇ<\C@fpIG]ۀ ,qC/ũ\{&}zmY،Im;|Kȹ.;68Qt'p|Ś/d{IWi3l8qE\}C7yI3Q_Բeݧj #m/v_pN[(rT7YNT{3RWyG 51Km>Zηg:HՂ(KTnxa[N6 Pq w #&br}x0Aih/@OFZ\btDd;0a E{4Ȑ(g ځf8B}{$cp憬]Ww x;ʓ{Lc+@5?S}G%8;":ʭלNe^R0A_AJI|Y73 Ш]ZC^vfq[  ?pC#S}SL;/Zm<)b2S?Ժuv06j=u:V(M6nYzZYo/-O#jh%0 ?~plʲg-t[1T>/ka x2 {runmO7@y-(Y{Pbq+"nMM@v:ŞBA?S}rXOǦ:帅(-rim7iKElbA❳{ Ġww 8ln.b /SwqҀ}nVdq]lܩ=!;=%; r.}4u JfnLwٝ{h E QָCO%tj}5ē-/̴߮?]>g׾\F#X©!UlmBiҺGTn\;>ZS)c[HU9*i`F=]a8)A 2'18QYP_)0S\ =7Vl38v1_q.ry2XSJA^bQY=:eDPpNH*5'0ES>9ɆҨ?{ɬ6&8?MNݜ >mz9,S.|iO&^ 26)iH̲H\dg;,S]'1!qKg=2ɂHH%3f<*H1*w˒wYvxHYDإ!rTlطi+?6 ƒ6><\{ 7jOlH (IQL͂>ps1(Ry gh#ѹ1I%j\0h:pR{@b JpxX L.$6]nj|${.EA}J .WJ<{R]d,O}DD2@Ĉ q8!䉱% 2bԭ8 VPQCA4*x.2˫9h3A :iQ?z1Z)?62N#imT_Q٪U GYׇ1 gu>tT#|u/dDrVÕOUIƕb'`ZHx&S%2]8)kl2HPs"O:2I9ۆ\ IzT^,1 ORbmծvp،)sr1lqSͪo ?C`p8U쌥+uDr:#tv `cB l)qXqz׃:TʰB2"gB?<)ktMZ)!EHQ]SE(Ib盭6Ȫ$F2UGZT4γJkfhB<]{*FKGj3 !D7,jH5;xMz\SUtjZp'BK+fWx~}Hc# lU})y0-g^At&js$.i$EA'z:RshCMh*wd+ `w:4Fc3)7 t`㼴'Ť(L\ҵP>s89{j3Bpo[s'Qpg ]Z΅&Q<0ֵ6oJ$j^#T]xҝi703ttFs gu  tAO#=Iz"ӧBfb~x ,/m3q.j+ȵP:ά>Yrpe]/3>^ zꂪimboQtdg:Yg:_c3hά"5n$F͐C[V1Xf)N=Žΐ>Cqzդ@&| zB?=V&Z|O=sF7mԀ\-wX4rPшYtFdQ<x]e()0hͼb#ug3gM\1NOx2-i~Q P;FyU;>5ҎQ=)L*!C&dMxcѡFc?fVU RӵYueCx.7 F8SyynlNBڑb1 Z(UM/qziVY8I,o#uxNu.\гsIĪ';]8ǁlV52oLwLJׯCi9G-Eֵ/esqI㍵iǼ/їھLs;]&Mo-*7zdt:\>_x=X~'D(γ/j"J/@Hʺ $5p:x0vFQAZW |0ŋ0=>TCrQ[&{H:J Nmad MI fal"9tQY9pn5y6oӰ(< EQOيpи{Q~Qi|a,qHSͬ@qFbD%]J~\Ycz`r %-RF/D@ Nu M#GFS '; *8 LP8=|PȊCѾq%fN]>f 0aG2,I!avTZZ^G&/χx(ƴ0lo^BC9UQ2_/PjZ.Ũ3~4!3TD &A5X?P J5IrC8n <&/-0ts22"R@'dX€"+#~Q`cd+&qC^FYĎh ;IC<&(u‰8Tt9.Zh:ߌ3^jxֺ'<1y8E2-Qw>SHnIJ["?4jx+SH_ ^֏.DJ!Ü2y "ã13VA1aQ?8?nA,Ö9!̙(:6,(l 2񔥑 0Y13E:qd잠l`ߒ)N7ɟZLQ$;Jc4Xb, 'BFq)~:*p),D70AcQ >a (4kȬv~8FO1v6>Pc+Tx*bs' ~ ebð >ohIk2W/m32.\#MkO3v=UG@}]6{)M>d #Sޥb"Y \BF~+h*^S2QP S73JUݘi ^XXB&En !GMi:ܩ ^mv`zDy6SzB 9Wc"$~IyRU. 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Oxr-0=-zFv jÑMBq\Czӆ/D[2sRvQ"ܧˈ6/S-}:l(;kvS<4 lݝC@Cbw 0pӅj9[$}T8;'EY#*Bq"R,:kaCB zG->- "#)dN)JƇ endstream endobj 268 0 obj <>stream JFIFHHC    #%$""!&+7/&)4)!"0A149;>>>%.DIC;C  ;("(;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;v"K !1"AQ2Uaqt46#BRs35b$TCr ?~S_i:M%sQQ)v4FqiЫ_{vT54 Lc/㊮W#\YPH:1w'o8g[œIrMVي 1I}b" """ """ """ """ """ """ """ """ ""+_hK_YF28v WK~ܸ,Zz)Cg$P@3ey>/ $;9tQ' W"dl~D@DDD@DDD@DDD@DDD@DDD@DDD@DDD@DDD@DDMQt!U55KVa~H g; %t{s# AVAGUM\}!O0[Ӳp.#oqUa(yruݲܳ+Dٞo-# )&豹9׫M첵OյÏڳِ;ϨɳϳG1nƌtaH\Ӹ+דoQβ,189!ǽѴ'گڱ%IјHْϓ<6 o?*%M$уqѧI;osQ8ή?pP\d4!i iY 6 ѴQjʏPNt@f\3Zq3+UZٙ,,/{8̒B >OYOz-kw:mUʫuYFɜLJi9c$l{**ۄf;`Rߨ`4 ѴO'8_+w;%]ʮHl9t\3ŔJGUCWA 9G"AFx6*`k94 E2j}SDDD@DDD@Erye5ѵ ;=${b$Q!=샬Z7ڪC 2wxXRހd!dTe)𸁆.a vd?Z ;P9rFI`gz-S)YNz'F{MEIN*'Q .׹h\AS | `Mmxx۹דF<6 -5dM<sۋQ tc>}<=gm??i OYOz*(wF<6 viL2@-h9u@Y;LNw8Pkff6|4p٭NnP #O{=kΪ4Stǐs@j;7)cpԆV(\ 9i۬2F7%bbn=gm?; tFm`YNz'FQ\MܨEK}2Y%Ɛ09$d:_'y=gm?UX䎶H4H ${wrsj!tO"ѱg5gQ-]ѴO'd msNZ3 oW'$Y U[%,2 Q;i=!HeObOYOz/xDrR,3̀Ai!cb :Bʦm62O>G?iOYOTq%$ձR;L0Wc\IC6p9"_6wPs?(4m,k /8}GMQV: G$ñ--" }Aky-Ij QTxitfi$chR eRS8\{I$Xx"o7{ sutԌFG j+b lG;F@Y%I_NjKku08#=];u-Gm0tu;s0;IϑAIFeI!詇H݂N9;؂:%Mں57$ 57q;T˅gW T2;T`;97cs- nBn{^00}`VUQo|sLvI;Cdlqߐ)j@TLt`. \ KWF2 dz[A""\+/b~^prpg GiuIv[rڨ慬| {fJV ni6be%. ;ΜV7|kuQg|uvn@$FdAD fHRDD+n%q0ISQFC'lʶ9QjIghu;烃0xA[頴6yTJ**.$l9qS÷+5$Ms*l/K0y-eM׆fl`oEIׂP w{H9uQQ:ںFH߳\2`lFN6pGӃ3j! ߑpy K+i/n`,/,V:QG e:r\G7- ;I _~:)2(j:Vkg ?96A[xRježz:VA\~Ny~k 8~**_J5|Mksݸ.P/` Xa˜rL-'|lpv;+KJ!,eƴv{qhrin=oa]h44[DzI Z4Kr+U:ic.{K^nx8b |Iг|' i𞓟/7u"U:xʺI ژjz75Ѵ7IC$g#l/{4vw95t5q| eբ 9*j :􆦖)f5r;W UX))5nzfچpFB؆Is'{v(utQ1:֌ ;}j oPP8:pr%ƬV"" """ """ ""yʚy)"" """ """ ~r?-*)5&oџa휞['2 t'8TJuƊZjj*f9gD~ dxmi4Ta$;$U]omf_X:O6 US(4=^dR=_>gxʂ$차ٌ8d---*<Acqg!uLګj?MLګj?j]+=u(wRZl {CZ# ) E>Lnjѱ١?´Cұl7:.jܲ8;*ܥs<bvp-4Dj1Ũjqݹ }kbtpGaaiRX-Kcs\5;nSAZ̰\)eKZ?=V7A݌6C$=8 Yh0~ X4=x*OoV9+Y @XPߤ22ӌ"Gش ؃n( b8Ɩ^ ȯ8_4O_4A"p8mC$ [LSXnFy-ިPc=pK&1c5 ˘#DDA}4NӜ}KO=/wp͹8mDg {#n5〽(G~|C]cIr%QnX,@io]h^-0hM4|24x {b}y{n kA.'xG:*;-AC[cNێNyԱHF籎,ުKph!u=MUK8ysEk H# F3AMF nFp^CAzJi*)! cS?c-ڎ(Njd/Ȑ wZ\/eR1CZ@ qD@DDD@DDD@DD2۽52۽SDDD@DDq[RNb .x#K 3#'>cZ7 :7QAWHcOTA:jAG3j -|M543fV7:a.WԺKfe-Mw4MFjgB&܏ ~r?*H=Q%֚r1^3AQAIVAW7s oR}a7SG<gP'$ mqȬWiH69=7'ibGSL8$$= Zm^:mW ;$@DDk(i7еƒ:ayipl-j :B]OMnwjw?Zѻ[f|mL`e>x3w;pq .d7?w:`IQ{}ѲdJ4@#c푂ӎUi9)]3hda#Ďcp`mLrCQ;t# g iV Ax,d]$}?c[$꒚#؈>i[tUw,cZ `5TLګj?MLګj?Kmxi-i8ڨ.7{+SIPi-Tt {&f 07vՠƬmYQoub堔N߄҂ uqRE4$tFX;:8?ZX(!mD c1$N-p}ag@Z_w+mj]+=C 7 :C 7 :" !4 kH :yˈ v{e DY)ҟV /Sku?bi1$inoH#e5 Y8z]nHvJ{}uƚYI+j:w4 u1Jh:C%LîK8n IK4\n.8^ZC]ۂ,V(#|qRA${[ަ\hjs.9:rd` Gk]v9lQh=H5mI=- h44 9Ç>k%m1\& C[1$dNSRI#_K#5ؐr֍;9]k RWI4vt@qgǬ`4"}pkǥtn`'\j$jqͪ}UãoIQ;#:[j" """ """ ~U~{#>U~{#/YOvma󺜵. xp$w#-{Z9# 9:I n)[Ul~ʞZJTJ 4[_{NbSYX{Q;f|'%$;?{X$1Y3;Ot 3VWi*`> aէ7]Um7 9)*r .-# 7T#jAMfsI#N۠lb3ܦ$sLÉ r99d7+o=/z:-S48I$w$I>[=/QZw {k`餁Z=cn"5X;*ttlsy$wy 0a`}, # <Έ + MIMGGKO ?{sihmGt3U ,ue eysZ;FAA6v Yc5i{d僰guttp>6}d,Z4Xؾ eϷ{?*jeϷ{?  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A.-ҫ >mYu Z?62K_5|WiEn.p+bDk:yx`3N5 66U Qp%o ( YYT2[0pa`~HiMP]וXᅗ$LWIձ|-H~c}7jX-#*}%j ^Xs#} 㖌"9eaܮ5úFg=v"yM+D&0;C*+)cue:}˲N1]u-i~#ȍLH~T-6S=Jپ=/cXn⋗MɐX]rr4e\ɘ[nj:*@O%nQ'mrj_F1i-=d O$R{V+$a)q%@fQ7|,KB3k?,1N$ 6&0A LnbC2dk(v 1|m!WkªXU,݃rc *u0a 7^\zXJ'[͑_zI R!Qd٫Ϥ؅ALm3J-ν'npaCP-COrܾ͂9\j'D*+]ϰk^[ J^M L55T7ma==|\ r3$GuÜxɑl{ u;K}"<2&㇬pOʁH!ICګ6SjFLPQ <\c 8Ꭷb,ǜ` 8=џĐiLsLG0t?gFfT }s}rtq-/}"G%eS[xV{$:]b)X>3Ҏڽ|hXs:=~rQ5OdLI(Jؽ]s fX"FbPCt )Dπ^B &sZR>G<\>ACK~L@lș5vqz7$SS~(XV 6?ƂÁe =t&,<t0gunmgxNZpقs Jܭ&f Ph>\7# =|_]R(WHZ㐠^I  5Дi.Lj{W_"'(^CV%Ѭt{E#hihb'4~k]E(*f>3U[ L״B=׌5񺄲xLp))&6|nF=jkfv&LdVUr2\ftA KTHCRIK=1qgG"o.nũԃ2lg iYIL ̰|Xʰ93{:>,}h B$q`U>riSE}Py&pAr;*_vKuwC؏yi-=flli:# ]BBJ$pe=9:o+KhmGw:K .Iƪ"ZU=tV(;zo<5@||daoDR2[Uɔ@jy xD]ջwߍtӪ<錏p}U58ΡRhUXyz\%V$ BZ͹!1.rk];J -qT1;Z"3z!dEP~=&6u̚\ص8\b~0IerѲA.iDN VF&0fE(죇/lv[#Bwe&OcO٭ ZU ٤s*6 S%%@5; J&$=zwI67UxL}?-扯j T^sPɑ:vpKL$[ujפt*9iOHc g3Fk_ĵq/)y<džnJf=oW}@m l:3VMv[nKYUlѷL ҳ[A֬8i% iWKLZ:kDo!y2Q5* hAt"AM@6!Vx^;9X-w<-ʑ#<$DP(Ɠ`9Uz2G 7$%JɔUJKM4wA:aH{ 5Fe0^NjiN2,$ &S:zUOxglRnoȡ $\#w_· Z$ǚ)ݔ :+/^,shwF&&uFh)ao6 w6%hvSs瞶_mz<Bw+'ӯ?0yHu⛃WDoΜ|d̉~N\t(KDϖ|> 럜Cg50h=NCg>fNg _)~_upl~8we_i50neѻ KnyF QA EY9Fء[Ƿ]!+al7~f]/Y7HY?4_hO|O}>?Nlc4}D& rkca8zƿ*k~oA=ȿ ߃5/x@&x~A endstream endobj 395 0 obj <>stream xj0B٠d7%]B)lwCDF6lfxR?h7M%S6^*nY%-LYDQn,޹~)aPU9v *d\nIߏ塞Jk7//}ÅxrdL 2A& 係̢I-{G١ endstream endobj 396 0 obj <>stream x|ңȲbyBBb(fWE?RB̬OU{zqd)DxOG̭&Y7Y[i&]|X '\_~U[Ńfʺ7֏ ~~܆߾y6?roκft774M7"0(+Jñw_.Jpoah~tWeYA~-~z_/"qvY;dMq_|W~{[T0(WןwYu?M17ݶ霦)߿'(<b~E_1Aw@yUPYٿregw},m[; t0CNY41zN[?5Ϻ%MW{?}~Y_0Wn] =0NȮe^u#Eip=?|c't=!]`JɉΫC ^†; qfQ^5kQ a cm0qCifO߻ mspӣ'//F̓]./9 X8_~0)qg"m]evdm@.7xuDZm0l$&dE8ꭘnfwgI8H>$v\uFҰeѕmRq7B$]K6[:P(M!&,ԯۂ<6Tޓ-,I5oUjƾ󩩱|2s_-0!T7[6RWOX@t&vwRpVk]hm+udYɽEE;\˵}D kMC1Α268ڥWE] c3!T\$3jǰEMn7j4>04axcӍޝ/_?[$)5v2?W۾𳾱6<ف}8k|Ѓ*7ޒFB 2r d jR{{kqaՓN eWs; xbVI&$Mq\F=bKlìYZY3݆2Fyi歮ٱh2'@;Zvu'y;. 2vuZ/;;H`qϺWr! DG86fK󪾾|cB@ɑZlaٰ3mA֌ yrԲ8ZMG::i2v@Wo䯓V0j*MȵI]s_ Ⱦ\gpV";gYikSflErxksi8!U^ڛУQ4alr'K*=專fˡ"Pɒ6Ç!RQ:d* ,a?"N-CD>^iCk-]Wj6SP-c1(ލd WeV(6O;4Qwq ͌#n đtkT IssfADۛA{7p,'jx<}zPKz7]294f;m˪jnlҽJ^!fvGPvB^܆% [RGGP5v펛/o L{"J)8o'l uA Xy^@ 6Qoʃ`zj$hΗmh<7⻶N(11goC:Y! d9H Vs{х|tBsaZq¿^Fv:!fؓ Y.O~?W=-* RH3yꘓ9>$1yy̾~~qfC]\с8JK:(2/mXsKZflkdБ%6R'2]%u0bR}JN_7l K;."jI%Yrv sR(4ra!Y57p[vf;As2b'A_O_W{6~U/ӻ } scŴ[kwhl#1WwpzE@n]%\zKT=eVu"$x49>2p!ڱ\صEۂݗd@O{-wUOsGS~%]%}zv-E#@z=y@X^)UntPaqlÒW*$>9ݬ{I;ј~*R$ 3iu&HF2uG FAh <= M}b><k pR⪓gP˼Ϙ/)Fyfc|"F_F!nI# GPOXk`;N'QWυr y̅N 'Aq/_3OΆ΄^6#9XaP6:62xx䏄 '0cɫ`q`Qa]>Hl9ۢ;p* YìwD'q_uϦ 4Ez@-Ua;-_&dp„! 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